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Latest progress in numerical simulations on multiphase flow and thermodynamics in production of naturalgas from gas hydrate reservoir

Lin ZUO, Lixia SUN, Changfu YOU

《能源前沿（英文）》 2009年 第3卷 第2期   页码 152-159 doi: 10.1007/s11708-009-0017-x

摘要： Natural gas hydrates are promising potential alternative energy resources. Some studies on the multiphase flow and thermodynamics have been conducted to investigate the feasibility of gas production from hydrate dissociation. The methods for natural gas production are analyzed and several models describing the dissociation process are listed and compared. Two prevailing models, one for depressurization and the other for thermal stimulation, are discussed in detail. A comprehensive numerical method considering the multiphase flow and thermodynamics of gas production from various hydrate-bearing reservoirs is required to better understand the dissociation process of natural gas hydrate, which would be of great benefit to its future exploration and exploitation.

关键词： numerical simulation     natural gas hydrate     dissociation     thermodynamics     multiphase flow    

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Life cycle assessment and economic analysis of HFC-134a production from natural gas compared with oil-basedand coal-based production

《化学科学与工程前沿（英文）》 2022年 第16卷 第12期   页码 1713-1725 doi: 10.1007/s11705-022-2210-y

摘要： China is the largest producer and consumer of HFC-134a (1,1,1,2-tetrafluoroethane) in the world. Coal-based route is mainly adopted to produce HFC-134a, which suffers from large waste and CO2 emissions. Natural gas is a low-carbon and clean energy resource, and no research has been found on the environment and economy of producing HFC-134a from natural gas. In this study, CML 2001 method was used to carry out the life cycle assessment of natural gas (partial oxidation)-based and natural gas (plasma cracking)-based routes (abbreviated as gas(O)-based and gas(P)-based routes, respectively), and their environmental performances were compared with coal-based and oil-based routes. Meanwhile, considering that China is vigorously promoting the transformation of energy structure, and the application of electric heating equipment to replace fossil-based heating equipment in industrial field, which has a great impact on the environmental performance of the production processes, the authors conducted a scenario analysis. The results showed that the gas(O)-based route had the most favourable environmental benefits. However, the gas(P)-based route had the highest potential for reducing environmental burdens, and its environmental benefit was the most favourable in scenario 2050. Additionally, the economic performance of the gas(P)-based route was significantly better than that of gas(O)-based and coal-based routes.

关键词： life cycle assessment     economic performance     HFC-134a     natural gas     oil     coal    

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Production of hydrogen from fossil fuel: A review

《能源前沿（英文）》 2023年 第17卷 第5期   页码 585-610 doi: 10.1007/s11708-023-0886-4

摘要： Production of hydrogen, one of the most promising alternative clean fuels, through catalytic conversion from fossil fuel is the most technically and economically feasible technology. Catalytic conversion of natural gas into hydrogen and carbon is thermodynamically favorable under atmospheric conditions. However, using noble metals as a catalyst is costly for hydrogen production, thus mandating non-noble metal-based catalysts such as Ni, Co, and Cu-based alloys. This paper reviews the various hydrogen production methods from fossil fuels through pyrolysis, partial oxidation, autothermal, and steam reforming, emphasizing the catalytic production of hydrogen via steam reforming of methane. The multicomponent catalysts composed of several non-noble materials have been summarized. Of the Ni, Co, and Cu-based catalysts investigated in the literature, Ni/Al2O3 catalyst is the most economical and performs best because it suppresses the coke formation on the catalyst. To avoid carbon emission, this method of hydrogen production from methane should be integrated with carbon capture, utilization, and storage (CCUS). Carbon capture can be accomplished by absorption, adsorption, and membrane separation processes. The remaining challenges, prospects, and future research and development directions are described.

关键词： methane     catalytic conversion     natural gas     hydrogen production     CCUS    

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Key issues in development of offshore natural gas hydrate

Shouwei ZHOU, Qingping LI, Xin LV, Qiang FU, Junlong ZHU

《能源前沿（英文）》 2020年 第14卷 第3期   页码 433-442 doi: 10.1007/s11708-020-0684-1

摘要： As a new clean energy resource in the 21st century, natural gas hydrate is considered as one of the most promising strategic resources in the future. This paper, based on the research progress in exploitation of natural gas hydrate (NGH) in China and the world, systematically reviewed and discussed the key issues in development of natural gas hydrate. From an exploitation point of view, it is recommended that the concepts of diagenetic hydrate and non-diagenetic hydrate be introduced. The main factors to be considered are whether diagenesis, stability of rock skeleton structure, particle size and cementation mode, thus NGHs are divided into 6 levels and used unused exploitation methods according to different types. The study of the description and quantitative characterization of abundance in hydrate enrichment zone, and looking for gas hydrate dessert areas with commercial exploitation value should be enhanced. The concept of dynamic permeability and characterization of the permeability of NGH by time-varying equations should be established. The ‘Three-gas co-production’ (natural gas hydrate, shallow gas, and conventional gas) may be an effective way to achieve early commercial exploitation. Although great progress has been made in the exploitation of natural gas hydrate, there still exist enormous challenges in basic theory research, production methods, and equipment and operation modes. Only through hard and persistent exploration and innovation can natural gas hydrate be truly commercially developed on a large scale and contribute to sustainable energy supply.

关键词： natural gas hydrate exploitation offshore     diagenetic and non-diagenetic hydrate     solid-state fluidization method     dessert in enrichment area     three-gas combined production on gas hydrate abundance    

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Phylogenetic diversity of NO reductases, new tools for monitoring, and insights into NO production innatural and engineered environments

《环境科学与工程前沿（英文）》 2022年 第16卷 第10期 doi: 10.1007/s11783-022-1562-3

摘要：

● 548 representative nor genes were collected to create complete phylogenetic trees.

关键词： N2O     Greenhouse gas     NO reductase     NO dismutase     Primer     Crystal structure    

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Removal efficiencies of natural and synthetic progesterones in hospital wastewater treated by different

《环境科学与工程前沿（英文）》 2022年 第16卷 第10期 doi: 10.1007/s11783-022-1558-z

摘要：

● The concentrations of 61 progesterones in HWW, PFTE, SBTE were evaluated.

关键词： Progesterones     Hospital wastewater     Primary filtration treatment effluent     Secondary biological treatment effluent     Disinfection process    

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天然气水合物资源勘探与试采技术研究现状与发展战略

付强,周守为,李清平

《中国工程科学》 2015年 第17卷 第9期   页码 123-132

摘要：

天然气水合物是甲烷等烃类气体与水在高压低温条件下形成的笼形化合物，俗称可燃冰，将有望成为继页岩气、致密气、煤层气、油砂等之后的储量最为巨大的接替能源，主要分布在北极冻土带和沿海大陆架300~3000 m水深的深水区，初步估计其资源量为全球含碳化合物的两倍，其中约95 %储存在深海区域；与此同时，深水浅层弱胶结水合物的无序分解等潜在工程地质灾害、温室效应等也已引起世界各国的高度重视，因此，天然气水合物资源安全高效开发和环境风险并重，成为当前世界科技创新的前沿。本文回顾了国内外天然气水合物资源勘探和试采技术研究进展，在此基础上，针对我国海域潜在目标区以及我国已经获取的天然气水合物样品的相关特性，提出了我国天然气水合物资源勘探开发技术方向。

关键词： 天然气水合物；勘探与试采；储量巨大；研究现状；发展战略    

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Characterization and catalytic activity of soft-templated NiO-CeO

Luciano Atzori, Maria Giorgia Cutrufello, Daniela Meloni, Barbara Onida, Delia Gazzoli, Andrea Ardu, Roberto Monaci, Maria Franca Sini, Elisabetta Rombi

《化学科学与工程前沿（英文）》 2021年 第15卷 第2期   页码 251-268 doi: 10.1007/s11705-020-1951-8

摘要： Nanosized NiO, CeO and NiO-CeO mixed oxides with different Ni/Ce molar ratios were prepared by the soft template method. All the samples were characterized by different techniques as to their chemical composition, structure, morphology and texture. On the catalysts submitted to the same reduction pretreatment adopted for the activity tests the surface basic properties and specific metal surface area were also determined. NiO and CeO nanocrystals of about 4 nm in size were obtained, regardless of the Ni/Ce molar ratio. The Raman and X-ray photoelectron spectroscopy results proved the formation of defective sites at the NiO-CeO interface, where Ni species are in strong interaction with the support. The microcalorimetric and Fourier transform infrared analyses of the reduced samples highlighted that, unlike metallic nickel, CeO is able to effectively adsorb CO , forming carbonates and hydrogen carbonates. After reduction in H at 400 °C for 1 h, the catalytic performance was studied in the CO and CO co-methanation reaction. Catalytic tests were performed at atmospheric pressure and 300 °C, using CO/CO /H molar compositions of 1/1/7 or 1/1/5, and space velocities equal to 72000 or 450000 cm ∙h ∙g . Whereas CO was almost completely hydrogenated in any investigated experimental conditions, CO conversion was strongly affected by both the CO/CO /H ratio and the space velocity. The faster and definitely preferred CO hydrogenation was explained in the light of the different mechanisms of CO and CO methanation. On a selected sample, the influence of the reaction temperature and of a higher number of space velocity values, as well as the stability, were also studied. Provided that the Ni content is optimized, the NiCe system investigated was very promising, being highly active for the CO co-methanation reaction in a wide range of operating conditions and stable (up to 50 h) also when submitted to thermal stress.

关键词： soft template method     NiO-CeO2 catalysts     CO and CO2 co-methanation     synthetic natural gas production    

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Research on the theory and application of adsorbed natural gas used in new energy vehicles: A review

Zhengwei NIE,Yuyi LIN,Xiaoyi JIN

《机械工程前沿（英文）》 2016年 第11卷 第3期   页码 258-274 doi: 10.1007/s11465-016-0381-2

摘要：

Natural gas, whose primary constituent is methane, has been considered a convincing alternative for the growth of the energy supply worldwide. Adsorbed natural gas (ANG), the most promising methane storage method, has been an active field of study in the past two decades. ANG constitutes a safe and low-cost way to store methane for natural gas vehicles at an acceptable energy density while working at substantially low pressures (3.5–4.0 MPa), allowing for conformable store tank. This work serves to review the state-of-the-art development reported in the scientific literature on adsorbents, adsorption theories, ANG conformable tanks, and related technologies on ANG vehicles. Patent literature has also been searched and discussed. The review aims at illustrating both achievements and problems of the ANG technologies-based vehicles, as well as forecasting the development trends and critical issues to be resolved of these technologies.

关键词： adsorbed natural gas (ANG)     adsorbent     adsorption theory     conformable tank     natural gas vehicles (NGVs)    

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A novel methodology for forecasting gas supply reliability of natural gas pipeline systems

Feng CHEN, Changchun WU

《能源前沿（英文）》 2020年 第14卷 第2期   页码 213-223 doi: 10.1007/s11708-020-0672-5

摘要： In this paper, a novel systematic and integrated methodology to assess gas supply reliability is proposed based on the Monte Carlo method, statistical analysis, mathematical-probabilistic analysis, and hydraulic simulation. The method proposed has two stages. In the first stage, typical scenarios are determined. In the second stage, hydraulic simulation is conducted to calculate the flow rate in each typical scenario. The result of the gas pipeline system calculated is the average gas supply reliability in each typical scenario. To verify the feasibility, the method proposed is applied for a real natural gas pipelines network system. The comparison of the results calculated and the actual gas supply reliability based on the filed data in the evaluation period suggests the assessment results of the method proposed agree well with the filed data. Besides, the effect of different components on gas supply reliability is investigated, and the most critical component is identified. For example, the 48th unit is the most critical component for the SH terminal station, while the 119th typical scenario results in the most severe consequence which causes the loss of 175.61×10 m gas when the 119th scenario happens. This paper provides a set of scientific and reasonable gas supply reliability indexes which can evaluate the gas supply reliability from two dimensions of quantity and time.

关键词： natural gas pipeline system     gas supply reliability     evaluation index     Monte Carlo method     hydraulic simulation    

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efficient utilization of coal resources: The polygeneration system of a combination of the gasified coal gasand the pyrolyzed coal gas to form the synthetic gas

Kechang XIE, Fan LI

《化学科学与工程前沿（英文）》 2010年 第4卷 第4期   页码 383-384 doi: 10.1007/s11705-010-0526-5

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Hollow-fiber gas penetration electrodes efficiently produce renewable synthetic fuels

《能源前沿（英文）》 2022年 第16卷 第5期   页码 700-705 doi: 10.1007/s11708-022-0842-8

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A review on technologies with electricity generation potentials using liquified natural gas regasification

《能源前沿（英文）》 2023年 第17卷 第3期   页码 332-379 doi: 10.1007/s11708-023-0863-y

摘要： In modern times, worldwide requirements to curb greenhouse gas emissions, and increment in energy demand due to the progress of humanity, have become a serious concern. In such scenarios, the effective and efficient utilization of the liquified natural gas (LNG) regasification cold energy (RCE), in the economically and environmentally viable methods, could present a great opportunity in tackling the core issues related to global warming across the world. In this paper, the technologies that are widely used to harness the LNG RCE for electrical power have been reviewed. The systems incorporating, the Rankine cycles, Stirling engines, Kalina cycles, Brayton cycles, Allam cycles, and fuel cells have been considered. Additionally, the economic and environmental studies apart from the thermal studies have also been reviewed. Moreover, the discussion regarding the systems with respect to the regassification pressure of the LNG has also been provided. The aim of this paper is to provide guidelines for the prospective researchers and policy makers in their decision making.

关键词： liquified natural gas     cold energy     power generation    

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Mesoporous zeolites as efficient catalysts for oil refining and natural gas conversion

Jie ZHU, Xiangju MENG, Fengshou XIAO

《化学科学与工程前沿（英文）》 2013年 第7卷 第2期   页码 233-248 doi: 10.1007/s11705-013-1329-2

摘要： Zeolites have been regarded as one of the most important catalysts in petrochemical industry due to their excellent catalytic performance. However, the sole micropores in zeolites severely limit their applications in oil refining and natural gas conversion. To solve the problem, mesoporous zeolites have been prepared by introducing mesopores into the zeolite crystals in recent years, and thus have the advantages of both mesostructured materials (fast diffusion and accessible for bulky molecules) and microporous zeolite crystals (strong acidity and high hydrothermal stability). In this review, after giving a brief introduction to preparation, structure, and characterization of mesoporous zeolites, we systematically summarize catalytic applications of these mesoporous zeolites as efficient catalysts in oil refining and natural gas conversion including catalytic cracking of heavy oil, alkylation, isomerization, hydrogenation, hydrodesulfurization, methane dehydroaromatization, methanol dehydration to dimethyl ether, methanol to olefins, and methanol to hydrocarbons.

关键词： mesoporous zeolite     catalysis     oil refining     natural gas conversion    

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Accelerating the construction of natural gas system engineering in green smart cities

Xinhua MA

《工程管理前沿（英文）》 2019年 第6卷 第3期   页码 453-456 doi: 10.1007/s42524-019-0046-z

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标题 作者 时间 类型 操作

Latest progress in numerical simulations on multiphase flow and thermodynamics in production of naturalgas from gas hydrate reservoir

Lin ZUO, Lixia SUN, Changfu YOU

期刊论文

Life cycle assessment and economic analysis of HFC-134a production from natural gas compared with oil-basedand coal-based production

期刊论文

Production of hydrogen from fossil fuel: A review

期刊论文

Key issues in development of offshore natural gas hydrate

Shouwei ZHOU, Qingping LI, Xin LV, Qiang FU, Junlong ZHU

期刊论文

Phylogenetic diversity of NO reductases, new tools for monitoring, and insights into NO production innatural and engineered environments

期刊论文

Removal efficiencies of natural and synthetic progesterones in hospital wastewater treated by different

期刊论文

天然气水合物资源勘探与试采技术研究现状与发展战略

付强,周守为,李清平

期刊论文

Characterization and catalytic activity of soft-templated NiO-CeO

Luciano Atzori, Maria Giorgia Cutrufello, Daniela Meloni, Barbara Onida, Delia Gazzoli, Andrea Ardu, Roberto Monaci, Maria Franca Sini, Elisabetta Rombi

期刊论文

Research on the theory and application of adsorbed natural gas used in new energy vehicles: A review

Zhengwei NIE,Yuyi LIN,Xiaoyi JIN

期刊论文

A novel methodology for forecasting gas supply reliability of natural gas pipeline systems

Feng CHEN, Changchun WU

期刊论文

efficient utilization of coal resources: The polygeneration system of a combination of the gasified coal gasand the pyrolyzed coal gas to form the synthetic gas

Kechang XIE, Fan LI

期刊论文

Hollow-fiber gas penetration electrodes efficiently produce renewable synthetic fuels

期刊论文

A review on technologies with electricity generation potentials using liquified natural gas regasification

期刊论文

Mesoporous zeolites as efficient catalysts for oil refining and natural gas conversion

Jie ZHU, Xiangju MENG, Fengshou XIAO

期刊论文

Accelerating the construction of natural gas system engineering in green smart cities

Xinhua MA

期刊论文